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Real-space Imaging of Quantum Hall Quasiparticles

Jinghao Deng, Yiming Sun, Dimitri Pimenov, Takashi Taniguchi, Kenji Watanabe, Erich J Mueller, Xiaomeng Liu

Jun 23, 2026arXiv:2606.25036v1
cond-mat.mes-hall
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Scorecard· 5/16
9.5/10 impact

Abstract

Quantum Hall systems host emergent quasiparticles with unusual charge, spin, and statistics, such as fractionally charged anyons. Although transport measurements have revealed many of their collective properties, identifying and visualizing individual quasiparticles remain elusive. Here we use scanning tunneling spectroscopy (STS) to image quantum Hall quasiparticles in graphene. Within incompressible quantum Hall states, we observe spatial variation of Landau level energies originating from electrostatic potentials created by charged defects in graphene and the underlying hexagonal boron nitride (hBN). For surface and near-surface defects, the Coulomb potential lifts the degeneracy of Landau orbitals, producing discrete energy splittings that reveal Landau orbital wavefunctions. In quantum Hall ferromagnetic states, quasiparticles bound to defect potentials produce distinct spatial and spectroscopic signatures that serve as hallmarks of the presence and number of localized excitations. In the fractional quantum Hall regime at one-third filling, our theoretical calculations predict discrete spectroscopic changes associated with the sequential addition of localized anyons, with a three-anyon bound state quantitatively reproducing our experimental data at ν=5/3ν= 5/3. These observations establish spectroscopic fingerprints of quantum Hall quasiparticles and provide a pathway toward imaging and manipulating individual anyons in real space.

AI Impact Assessments

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Scientific Impact Assessment: "Real-space Imaging of Quantum Hall Quasiparticles"

1. Core Contribution

This paper reports the first direct real-space visualization of individual quantum Hall quasiparticles using scanning tunneling spectroscopy (STS) in monolayer graphene on hBN. The central advance is threefold: (i) imaging individual Landau orbitals through defect-induced orbital splitting at ν=2, (ii) detecting and distinguishing bound quasiparticle configurations in quantum Hall ferromagnetic states at ν=−1, and (iii) identifying spectroscopic signatures consistent with three bound anyonic quasiparticles at ν=5/3. The key conceptual insight is that charged defects in graphene and hBN act as natural nanoscale traps for quantum Hall quasiparticles, and that the number of trapped quasiparticles produces distinct, identifiable spectroscopic fingerprints—both in energy-resolved spectra and in spatially-resolved spectral weight.

This addresses a longstanding experimental gap: while transport measurements (shot noise, interferometry) have probed fractional charge and statistics indirectly, no technique had previously visualized individual quantum Hall quasiparticles in real space with the resolution needed to reveal their internal structure.

2. Methodological Rigor

The experimental methodology is exceptionally thorough. The authors employ careful tip preparation (charge-neutral tips verified via Haldane sash features), constant-height-setpoint protocols to ensure reliable spectral weight extraction, and multiple independent consistency checks. The observation of particle-hole symmetry between ν=5/3 and ν=−5/3 measurements (Fig. S11) provides compelling internal validation.

The theoretical framework is multi-layered and appropriate: exact diagonalization for integer quantum Hall states, and DMRG on the Haldane sphere for fractional states. The spectral function calculations use a sophisticated global Krylov method with ghost-state deflation, and results are cross-validated with an independent sequential excited-state approach. The agreement between theory and experiment is quantitative for the three-anyon bound state at ν=5/3, including both the energy sequence of orbital peaks and the screened Coulomb potential profile. Crucially, the authors demonstrate that zero, one, and two anyon configurations produce clear discrepancies with the data (Supplementary Fig. S10), strengthening the three-anyon interpretation.

The treatment of systematic effects is commendable. The tip screening model (metallic sphere with image charges), the chemical potential pinning mechanism explaining enlarged apparent gaps, and the careful estimation of subsurface defect depths all reflect deep understanding of potential artifacts. The explanation of why tunneling current—rather than gate voltage—controls quasiparticle occupation within incompressible states is a significant methodological insight for the STM community.

3. Potential Impact

Immediate field impact: This work establishes STS as a platform for detecting individual anyons, opening a fundamentally new experimental avenue in quantum Hall physics. The "quasiparticle microscope" concept—using the dichotomy between surface and subsurface defect spectra to detect bound quasiparticles—is elegant and broadly applicable.

Toward topological quantum computing: The authors explicitly note the possibility of combining visualization with tip-induced manipulation for anyon braiding demonstrations. If realized, this would constitute a qualitatively different approach to demonstrating non-Abelian statistics compared to interferometric methods.

Extensions to non-Abelian states: The methodology naturally extends to even-denominator fractional quantum Hall states (ν=5/2) and fractional Chern insulators in moiré systems, where non-Abelian anyons are theorized.

Materials science implications: The characterization of charged defect distributions in hBN—revealing their depths, charge states, and density—provides valuable information for the van der Waals heterostructure community, where such defects limit device quality.

Spectral weight sum rules: The demonstration that integrated dI/dV faithfully reproduces local electron/hole density, including the excess charge distribution of anyon bound states, establishes a quantitative link between STS observables and many-body wavefunctions.

4. Timeliness & Relevance

This work arrives at a critical moment. Recent interferometry experiments have provided evidence for anyonic braiding statistics, and there is intense interest in fractional Chern insulators in moiré materials. A real-space probe capable of imaging individual anyons fills a major experimental gap and could accelerate progress toward topological quantum computation. The graphene platform is particularly timely given its accessibility and the rapid improvements in device quality.

5. Strengths & Limitations

Key strengths:

  • Extraordinary spectral resolution revealing spin, valley, and orbital quantum numbers of individual Landau orbitals
  • Quantitative theory-experiment agreement for the three-anyon bound state, with clear discrimination from alternative configurations
  • Comprehensive treatment of systematic effects (tip screening, chemical potential pinning, setpoint artifacts)
  • Internal consistency checks (particle-hole symmetry, multiple defects, multiple filling factors)
  • The unified framework explaining quasiparticle binding conditions across different defect types and tunneling polarities
  • Notable limitations:

  • The number of bound anyons is primarily determined by defect strength rather than being externally controllable; the authors cannot yet tune between different anyon numbers at a single defect
  • For the +e defect at ν=5/3, the quasi-electron bound state identification is acknowledged as less reliable than the quasi-hole case
  • The theory assumes minimal m=0 wavefunctions for bound quasiparticles, while small skyrmions may be stabilized in some cases—a discrepancy the authors acknowledge
  • The spin-wave continuum predicted theoretically at ν=−1 appears as discrete peaks experimentally, suggesting additional physics (standing waves or disorder effects) not fully captured
  • Direct demonstration of fractional charge (e/3) of individual bound anyons—rather than the composite three-anyon state carrying charge e—remains to be achieved
  • Overall assessment: This is a landmark experimental and theoretical achievement that opens a new chapter in quantum Hall physics. The combination of atomic-resolution imaging, quantitative many-body theory, and clear physical interpretation makes this work exceptionally impactful. The pathway from visualization to manipulation of individual anyons, while speculative, is credibly outlined.

    Rating:9.3/ 10
    Significance 9.5Rigor 9Novelty 9.5Clarity 9

    Generated Jun 25, 2026

    Comparison History (31)

    Wonvs. Visualizing orbital magnetism in electron doped rhombohedral multilayer graphene

    Paper 1 achieves a historic milestone in fundamental physics: the real-space imaging of individual fractional quantum Hall quasiparticles (anyons). While Paper 2 presents highly impactful findings on chiral superconductivity in multilayer graphene, Paper 1's methodology for visualizing and potentially manipulating anyons unlocks direct pathways for topological quantum computing. The ability to observe discrete spectroscopic signatures of anyon bound states transcends traditional transport measurements, offering broader, paradigm-shifting implications across quantum condensed matter physics and quantum information science.

    gemini-3.1-pro-preview·Jul 24, 2026
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    claude-opus-4-8·Jul 24, 2026
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    gemini-3.1-pro-preview·Jul 24, 2026
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    gpt-5.2·Jul 24, 2026
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    Paper 2 provides direct real-space imaging of fractional quantum Hall quasiparticles and anyons, addressing a longstanding challenge with major implications for topological quantum computing and fundamental physics of anyonic statistics. The quantitative agreement between theory and experiment for a three-anyon bound state is a significant achievement. While Paper 1's q-SNOM is methodologically novel and technically impressive, Paper 2 tackles a more foundational, widely-sought goal (visualizing/manipulating individual anyons) with broader impact across condensed matter and quantum information communities.

    claude-opus-4-8·Jul 24, 2026
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    gpt-5.2·Jul 24, 2026